HW transcoding not working reliably

Does your Plex server have an active Nvidia GPU?
Based on your logs the server is trying to use that GPU and fails to do so. It’s not using the iGPU of your Celeron.
As a consequence there’s e.g. messages like this:

Sep 14, 2021 19:37:38.393 [2868] DEBUG - [Transcode] TPU: hardware transcoding: enabled, but no hardware decode accelerator found

PS: you seriously need to rethink your file naming…

TV Shows
  Marvel's Spider-Man
    Marvel's Spider-Man Specials
      Marvel's Spider-Man - 0x01 & 0x02 & 0x03 & 0x04 & 0x05 & 0x06 - Origin Shorts Introduction! & Origin Shorts Observation! & Origin Shorts Hypothesis! & Origin Shorts Prediction! & Origin Shorts Experimentation! & Origin Shorts Conclusion!.mkv

should be

TV Shows
  Marvel's Spider-Man
    Specials
      Marvel's Spider-Man - s00e01-e06.mkv
               -- OR --
      Marvel's Spider-Man - s00e01-e06 - Origin Shorts Introduction! & Origin Shorts Observation! & Origin Shorts Hypothesis! & Origin Shorts Prediction! & Origin Shorts Experimentation! & Origin Shorts Conclusion!.mkv